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https://doi.org/10.21256/zhaw-2790| Publikationstyp: | Konferenz: Poster |
| Art der Begutachtung: | Peer review (Abstract) |
| Titel: | Advanced characterization of polymer electrolyte fuel cells using a two-phase time-dependent model |
| Autor/-in: | Herrendörfer, Robert Schumacher, Jürgen O. |
| DOI: | 10.21256/zhaw-2790 |
| Tagungsband: | 16th symposium on modeling and experimental validation of electrochemical energy technologies (ModVal 2019) : book of abstracts |
| Herausgeber/-in des übergeordneten Werkes: | Krewer, Ulrike Laue, Vincent Redeker, Andreas |
| Angaben zur Konferenz: | ModVal 2019, Braunschweig, Germany, 12-13 March 2019 |
| Erscheinungsdatum: | 2019 |
| Verlag / Hrsg. Institution: | Technische Universität Braunschweig |
| Sprache: | Englisch |
| Schlagwörter: | Proton exchange membrane fuel cell model; Numerical simulation; Two-phase; Time dependent |
| Fachgebiet (DDC): | 621.3: Elektro-, Kommunikations-, Steuerungs- und Regelungstechnik |
| Zusammenfassung: | For polymer electrolyte fuel cells (PEFC) to become competitive, their operation in transport applications requires optimized performance, durability and costs. An indispensable component of this optimization is a detailed time-dependent characterization of PEFCs. For this purpose, several dynamic single-cell PEFC numerical models have been developed in the last 15 years. Here we present a new modeling approach with an advanced material parameterization of all governing time-dependent processes. This new modeling approach is based on the 1-D steady-state two-phase, five-layer PEFC model with a comprehensive material parametrization [1]. We further developed this approach by including the time-dependency of electron, proton, heat, dissolved water, gas and liquid water transport. Implementation in COMSOL allows for accurate spatio-temporal resolution and flexible model setups. We develop an improved electrochemical spectroscopy method by applying a sinusoidal perturbation of varying amplitude to the cell voltage. In contrast to (small-signal) electrical impedance spectroscopy, our model numerically solves for the nonlinear time-dependent response of the fuel cell, which enables us to retrieve information from large signals. We compute the response spectra at different operating points not only for electrical current density but also for dissolved water, liquid water, temperature and gas concentration and their gradients. These nonlinear response spectra serve for the development of improved model-based characterization techniques and fuel cell diagnostics. Acknowledgements: Financial support from the Swiss Federal Office of Energy (SFOE contract number: SI/501764-01) is gratefully acknowledged. |
| URI: | https://digitalcollection.zhaw.ch/handle/11475/16155 |
| Volltext Version: | Akzeptierte Version |
| Lizenz (gemäss Verlagsvertrag): | Keine Angabe |
| Departement: | School of Engineering |
| Organisationseinheit: | Institute of Computational Physics (ICP) |
| Publiziert im Rahmen des ZHAW-Projekts: | Neue Charakterisierungsmethoden von Brennstoffzellenstacks für den Einsatz im Automobilbereich (ACTIF) |
| Enthalten in den Sammlungen: | Publikationen School of Engineering |
Dateien zu dieser Ressource:
| Datei | Beschreibung | Größe | Format | |
|---|---|---|---|---|
| Poster.pdf | 2.18 MB | Adobe PDF |  Öffnen/Anzeigen | |
| poster_addon.pdf | 894.56 kB | Adobe PDF |  Öffnen/Anzeigen |
Zur Langanzeige
Herrendörfer, R., & Schumacher, J. O. (2019). Advanced characterization of polymer electrolyte fuel cells using a two-phase time-dependent model [Conference poster]. In U. Krewer, V. Laue, & A. Redeker (Eds.), 16th symposium on modeling and experimental validation of electrochemical energy technologies (ModVal 2019) : book of abstracts. Technische Universität Braunschweig. https://doi.org/10.21256/zhaw-2790
Herrendörfer, R. and Schumacher, J.O. (2019) ‘Advanced characterization of polymer electrolyte fuel cells using a two-phase time-dependent model’, in U. Krewer, V. Laue, and A. Redeker (eds) 16th symposium on modeling and experimental validation of electrochemical energy technologies (ModVal 2019) : book of abstracts. Technische Universität Braunschweig. Available at: https://doi.org/10.21256/zhaw-2790.
R. Herrendörfer and J. O. Schumacher, “Advanced characterization of polymer electrolyte fuel cells using a two-phase time-dependent model,” in 16th symposium on modeling and experimental validation of electrochemical energy technologies (ModVal 2019) : book of abstracts, 2019. doi: 10.21256/zhaw-2790.
HERRENDÖRFER, Robert und Jürgen O. SCHUMACHER, 2019. Advanced characterization of polymer electrolyte fuel cells using a two-phase time-dependent model. In: Ulrike KREWER, Vincent LAUE und Andreas REDEKER (Hrsg.), 16th symposium on modeling and experimental validation of electrochemical energy technologies (ModVal 2019) : book of abstracts. Conference poster. Technische Universität Braunschweig. 2019
Herrendörfer, Robert, and Jürgen O. Schumacher. 2019. “Advanced Characterization of Polymer Electrolyte Fuel Cells Using a Two-Phase Time-Dependent Model.” Conference poster. In 16th Symposium on Modeling and Experimental Validation of Electrochemical Energy Technologies (ModVal 2019) : Book of Abstracts, edited by Ulrike Krewer, Vincent Laue, and Andreas Redeker. Technische Universität Braunschweig. https://doi.org/10.21256/zhaw-2790.
Herrendörfer, Robert, and Jürgen O. Schumacher. “Advanced Characterization of Polymer Electrolyte Fuel Cells Using a Two-Phase Time-Dependent Model.” 16th Symposium on Modeling and Experimental Validation of Electrochemical Energy Technologies (ModVal 2019) : Book of Abstracts, edited by Ulrike Krewer et al., Technische Universität Braunschweig, 2019, https://doi.org/10.21256/zhaw-2790.
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