1. ZHAW digitalcollection
  2. School of Engineering
  3. Publikationen
  4. Publikationen School of Engineering
Full metadata record
DC FieldValueLanguage
dc.contributor.authorChiaia-Hernández, Aurea C.-
dc.contributor.authorGünthardt, Barbara F.-
dc.contributor.authorFrey, Martin-
dc.contributor.authorHollender, Juliane-
dc.date.accessioned2017-11-08T12:45:46Z-
dc.date.available2017-11-08T12:45:46Z-
dc.date.issued2017-10-25-
dc.identifier.issn0013-936Xde_CH
dc.identifier.issn1520-5851de_CH
dc.identifier.issn1520-5851de_CH
dc.identifier.urihttps://digitalcollection.zhaw.ch/handle/11475/1444-
dc.description.abstractThe significant increase in traces of human activity in the environment worldwide provides evidence of the beginning of a new geological era, informally named the Anthropocene. The rate and variability of these human modifications at the local and global scale remain largely unknown, but new analytical methods such as high-resolution mass spectrometry (HRMS) can help to characterize chemical contamination. We therefore applied HRMS to investigate the contamination history of two lakes in Central Europe over the preceding 100 years. A hierarchical clustering analysis (HCA) of the collected time series data revealed more than 13 000 profiles of anthropogenic origin in both lakes, defining the beginning of large-scale human impacts during the 1950s. Our results show that the analysis of temporal patterns of nontarget contaminants is an effective method for characterizing the contamination pattern in the Anthropocene and an important step in prioritizing the identification of organic contaminants not yet successfully targeted by environmental regulation and pollution reduction initiatives. As proof of the concept, the success of the method was demonstrated with the identification of the pesticide imazalil, which probably originated from imported fruits. This new approach applicable to palaeoarchives can effectively be used to document the time and rate of change in contamination over time and provide additional information on the onset of the Anthropocene.de_CH
dc.language.isoende_CH
dc.publisherAmerican Chemical Societyde_CH
dc.relation.ispartofEnvironmental Science & Technologyde_CH
dc.rightsLicence according to publishing contractde_CH
dc.subject.ddc540: Chemiede_CH
dc.titleUnravelling contaminants in the anthropocene using statistical analysis of liquid chromatography–high-resolution mass spectrometry nontarget screening data recorded in lake sedimentsde_CH
dc.typeBeitrag in wissenschaftlicher Zeitschriftde_CH
dcterms.typeTextde_CH
zhaw.departementSchool of Engineeringde_CH
zhaw.organisationalunitInstitut für Datenanalyse und Prozessdesign (IDP)de_CH
dc.identifier.doi10.1021/acs.est.7b03357de_CH
dc.identifier.pmid29067807de_CH
zhaw.funding.euNode_CH
zhaw.issue21de_CH
zhaw.originated.zhawYesde_CH
zhaw.pages.end12556de_CH
zhaw.pages.start12547de_CH
zhaw.publication.statuspublishedVersionde_CH
zhaw.volume51de_CH
zhaw.publication.reviewPeer review (Publikation)de_CH
Appears in collections:Publikationen School of Engineering

Files in This Item:
There are no files associated with this item.
Show simple item record
Chiaia-Hernández, A. C., Günthardt, B. F., Frey, M., & Hollender, J. (2017). Unravelling contaminants in the anthropocene using statistical analysis of liquid chromatography–high-resolution mass spectrometry nontarget screening data recorded in lake sediments. Environmental Science & Technology, 51(21), 12547–12556. https://doi.org/10.1021/acs.est.7b03357
Chiaia-Hernández, A.C. et al. (2017) ‘Unravelling contaminants in the anthropocene using statistical analysis of liquid chromatography–high-resolution mass spectrometry nontarget screening data recorded in lake sediments’, Environmental Science & Technology, 51(21), pp. 12547–12556. Available at: https://doi.org/10.1021/acs.est.7b03357.
A. C. Chiaia-Hernández, B. F. Günthardt, M. Frey, and J. Hollender, “Unravelling contaminants in the anthropocene using statistical analysis of liquid chromatography–high-resolution mass spectrometry nontarget screening data recorded in lake sediments,” Environmental Science & Technology, vol. 51, no. 21, pp. 12547–12556, Oct. 2017, doi: 10.1021/acs.est.7b03357.
CHIAIA-HERNÁNDEZ, Aurea C., Barbara F. GÜNTHARDT, Martin FREY und Juliane HOLLENDER, 2017. Unravelling contaminants in the anthropocene using statistical analysis of liquid chromatography–high-resolution mass spectrometry nontarget screening data recorded in lake sediments. Environmental Science & Technology. 25 Oktober 2017. Bd. 51, Nr. 21, S. 12547–12556. DOI 10.1021/acs.est.7b03357
Chiaia-Hernández, Aurea C., Barbara F. Günthardt, Martin Frey, and Juliane Hollender. 2017. “Unravelling Contaminants in the Anthropocene Using Statistical Analysis of Liquid Chromatography–High-Resolution Mass Spectrometry Nontarget Screening Data Recorded in Lake Sediments.” Environmental Science & Technology 51 (21): 12547–56. https://doi.org/10.1021/acs.est.7b03357.
Chiaia-Hernández, Aurea C., et al. “Unravelling Contaminants in the Anthropocene Using Statistical Analysis of Liquid Chromatography–High-Resolution Mass Spectrometry Nontarget Screening Data Recorded in Lake Sediments.” Environmental Science & Technology, vol. 51, no. 21, Oct. 2017, pp. 12547–56, https://doi.org/10.1021/acs.est.7b03357.


Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.