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Publikationstyp: Beitrag in wissenschaftlicher Zeitschrift
Art der Begutachtung: Peer review (Publikation)
Titel: Outstanding passivation effect by a mixed-salt interlayer with internal interactions in perovskite solar cells
Autor/-in: Yang, Bowen
Suo, Jiajia
Mosconi, Edoardo
Ricciarelli, Damiano
Tress, Wolfgang
De Angelis, Filippo
Kim, Hui-Seon
Hagfeldt, Anders
et. al: No
DOI: 10.1021/acsenergylett.0c01664
10.21256/zhaw-20648
Erschienen in: ACS Energy Letters
Band(Heft): 5
Heft: 10
Seite(n): 3159
Seiten bis: 3167
Erscheinungsdatum: 2020
Verlag / Hrsg. Institution: American Chemical Society
ISSN: 2380-8195
Sprache: Englisch
Fachgebiet (DDC): 621.3: Elektro-, Kommunikations-, Steuerungs- und Regelungstechnik
Zusammenfassung: Nonradiative recombination is a major limiting factor in obtaining efficient metal-halide perovskite photovoltaics. Here, a passivation treatment is developed by applying a mixture of a new ammonium salt, CF3(CF2)2CH2NH3I (HBAI), and a conventional formamidinium halide, FAX, on top of the 3D perovskite bulk film. The introduction of such an optimized passivation layer effectively suppressed charge recombination by passivating the surface traps of the 3D perovskite film, enabling a wellmatched energy alignment at the interface of perovskite/HTM, leading to a high power conversion efficiency (PCE) of over 23% from current−voltage (I−V) measurements and a stabilized 22.7% PCE, owing to a substantial VOC improvement (above 80 mV on average), coupled with an improved stability.
Weitere Angaben: This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Energy Letters, © 2020 American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://pubs.acs.org/doi/10.1021/acsenergylett.0c01664
URI: https://digitalcollection.zhaw.ch/handle/11475/20648
Volltext Version: Akzeptierte Version
Lizenz (gemäss Verlagsvertrag): Lizenz gemäss Verlagsvertrag
Gesperrt bis: 2021-09-14
Departement: School of Engineering
Organisationseinheit: Institute of Computational Physics (ICP)
Enthalten in den Sammlungen:Publikationen School of Engineering

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Yang, B., Suo, J., Mosconi, E., Ricciarelli, D., Tress, W., De Angelis, F., Kim, H.-S., & Hagfeldt, A. (2020). Outstanding passivation effect by a mixed-salt interlayer with internal interactions in perovskite solar cells. ACS Energy Letters, 5(10), 3159–3167. https://doi.org/10.1021/acsenergylett.0c01664
Yang, B. et al. (2020) ‘Outstanding passivation effect by a mixed-salt interlayer with internal interactions in perovskite solar cells’, ACS Energy Letters, 5(10), pp. 3159–3167. Available at: https://doi.org/10.1021/acsenergylett.0c01664.
B. Yang et al., “Outstanding passivation effect by a mixed-salt interlayer with internal interactions in perovskite solar cells,” ACS Energy Letters, vol. 5, no. 10, pp. 3159–3167, 2020, doi: 10.1021/acsenergylett.0c01664.
YANG, Bowen, Jiajia SUO, Edoardo MOSCONI, Damiano RICCIARELLI, Wolfgang TRESS, Filippo DE ANGELIS, Hui-Seon KIM und Anders HAGFELDT, 2020. Outstanding passivation effect by a mixed-salt interlayer with internal interactions in perovskite solar cells. ACS Energy Letters. 2020. Bd. 5, Nr. 10, S. 3159–3167. DOI 10.1021/acsenergylett.0c01664
Yang, Bowen, Jiajia Suo, Edoardo Mosconi, Damiano Ricciarelli, Wolfgang Tress, Filippo De Angelis, Hui-Seon Kim, and Anders Hagfeldt. 2020. “Outstanding Passivation Effect by a Mixed-Salt Interlayer with Internal Interactions in Perovskite Solar Cells.” ACS Energy Letters 5 (10): 3159–67. https://doi.org/10.1021/acsenergylett.0c01664.
Yang, Bowen, et al. “Outstanding Passivation Effect by a Mixed-Salt Interlayer with Internal Interactions in Perovskite Solar Cells.” ACS Energy Letters, vol. 5, no. 10, 2020, pp. 3159–67, https://doi.org/10.1021/acsenergylett.0c01664.


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