1. ZHAW digitalcollection
  2. School of Engineering
  3. Publikationen
  4. Publikationen School of Engineering
Full metadata record
DC FieldValueLanguage
dc.contributor.authorLee, Seung-Heon-
dc.contributor.authorLu, Jian-
dc.contributor.authorLee, Seung-Jun-
dc.contributor.authorHan, Jae-Hyun-
dc.contributor.authorJeong, Chan-Uk-
dc.contributor.authorLee, Seung-Chul-
dc.contributor.authorLi, Xian-
dc.contributor.authorJazbinsek, Mojca-
dc.contributor.authorYoon, Woojin-
dc.contributor.authorYun, Hoseop-
dc.contributor.authorKang, Bong Joo-
dc.contributor.authorRotermund, Fabian-
dc.contributor.authorNelson, Keith A.-
dc.contributor.authorKwon, O-Pil-
dc.date.accessioned2018-03-21T15:55:33Z-
dc.date.available2018-03-21T15:55:33Z-
dc.date.issued2017-
dc.identifier.issn0935-9648de_CH
dc.identifier.issn1521-4095de_CH
dc.identifier.urihttps://digitalcollection.zhaw.ch/handle/11475/4159-
dc.description.abstractHighly efficient nonlinear optical organic crystals are very attractive for various photonic applications including terahertz (THz) wave generation. Up to now, only two classes of ionic crystals based on either pyridinium or quinolinium with extremely large macroscopic optical nonlinearity have been developed. This study reports on a new class of organic nonlinear optical crystals introducing electron-accepting benzothiazolium, which exhibit higher electron-withdrawing strength than pyridinium and quinolinium in benchmark crystals. The benzothiazolium crystals consisting of new acentric core HMB (2-(4-hydroxy-3-methoxystyryl)-3-methylbenzo[d]thiazol-3-ium) exhibit extremely large macroscopic optical nonlinearity with optimal molecular ordering for maximizing the diagonal second-order nonlinearity. HMB-based single crystals prepared by simple cleaving method satisfy all required crystal characteristics for intense THz wave generation such as large crystal size with parallel surfaces, moderate thickness and high optical quality with large optical transparency range (580-1620 nm). Optical rectification of 35 fs pulses at the technologically very important wavelength of 800 nm in 0.26 mm thick HMB crystal leads to one order of magnitude higher THz wave generation efficiency with remarkably broader bandwidth compared to standard inorganic 0.5 mm thick ZnTe crystal. Therefore, newly developed HMB crystals introducing benzothiazolium with extremely large macroscopic optical nonlinearity are very promising materials for intense broadband THz wave generation and other nonlinear optical applications.de_CH
dc.language.isoende_CH
dc.publisherWileyde_CH
dc.relation.ispartofAdvanced Materialsde_CH
dc.rightsLicence according to publishing contractde_CH
dc.subjectNonlinear opticsde_CH
dc.subjectOrganic crystalde_CH
dc.subjectTerahertz wavede_CH
dc.subject.ddc530: Physikde_CH
dc.subject.ddc540: Chemiede_CH
dc.titleBenzothiazolium single crystals : a new class of nonlinear optical crystals with efficient THz wave generationde_CH
dc.typeBeitrag in wissenschaftlicher Zeitschriftde_CH
dcterms.typeTextde_CH
zhaw.departementSchool of Engineeringde_CH
zhaw.organisationalunitInstitute of Computational Physics (ICP)de_CH
dc.identifier.doi10.1002/adma.201701748de_CH
dc.identifier.pmid28589627de_CH
zhaw.funding.euNode_CH
zhaw.issue30de_CH
zhaw.originated.zhawYesde_CH
zhaw.pages.start1701748de_CH
zhaw.publication.statuspublishedVersionde_CH
zhaw.volume29de_CH
zhaw.publication.reviewPeer review (Publikation)de_CH
Appears in collections:Publikationen School of Engineering

Files in This Item:
There are no files associated with this item.
Show simple item record
Lee, S.-H., Lu, J., Lee, S.-J., Han, J.-H., Jeong, C.-U., Lee, S.-C., Li, X., Jazbinsek, M., Yoon, W., Yun, H., Kang, B. J., Rotermund, F., Nelson, K. A., & Kwon, O.-P. (2017). Benzothiazolium single crystals : a new class of nonlinear optical crystals with efficient THz wave generation. Advanced Materials, 29(30), 1701748. https://doi.org/10.1002/adma.201701748
Lee, S.-H. et al. (2017) ‘Benzothiazolium single crystals : a new class of nonlinear optical crystals with efficient THz wave generation’, Advanced Materials, 29(30), p. 1701748. Available at: https://doi.org/10.1002/adma.201701748.
S.-H. Lee et al., “Benzothiazolium single crystals : a new class of nonlinear optical crystals with efficient THz wave generation,” Advanced Materials, vol. 29, no. 30, p. 1701748, 2017, doi: 10.1002/adma.201701748.
LEE, Seung-Heon, Jian LU, Seung-Jun LEE, Jae-Hyun HAN, Chan-Uk JEONG, Seung-Chul LEE, Xian LI, Mojca JAZBINSEK, Woojin YOON, Hoseop YUN, Bong Joo KANG, Fabian ROTERMUND, Keith A. NELSON und O-Pil KWON, 2017. Benzothiazolium single crystals : a new class of nonlinear optical crystals with efficient THz wave generation. Advanced Materials. 2017. Bd. 29, Nr. 30, S. 1701748. DOI 10.1002/adma.201701748
Lee, Seung-Heon, Jian Lu, Seung-Jun Lee, Jae-Hyun Han, Chan-Uk Jeong, Seung-Chul Lee, Xian Li, et al. 2017. “Benzothiazolium Single Crystals : A New Class of Nonlinear Optical Crystals with Efficient THz Wave Generation.” Advanced Materials 29 (30): 1701748. https://doi.org/10.1002/adma.201701748.
Lee, Seung-Heon, et al. “Benzothiazolium Single Crystals : A New Class of Nonlinear Optical Crystals with Efficient THz Wave Generation.” Advanced Materials, vol. 29, no. 30, 2017, p. 1701748, https://doi.org/10.1002/adma.201701748.


Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.