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Publikationstyp: Beitrag in wissenschaftlicher Zeitschrift
Art der Begutachtung: Peer review (Publikation)
Titel: Experimental parameter uncertainty in proton exchange membrane fuel cell modeling - part II : sensitivity analysis and importance ranking
Autor/-in: Vetter, Roman
Schumacher, Jürgen O.
DOI: 10.1016/j.jpowsour.2019.04.057
10.21256/zhaw-17089
Erschienen in: Journal of Power Sources
Band(Heft): 439
Seite(n): 126529
Erscheinungsdatum: 1-Nov-2019
Verlag / Hrsg. Institution: Elsevier
ISSN: 0378-7753
1873-2755
Andere Identifier: arXiv:1811.10093
Sprache: Englisch
Schlagwörter: physics.app-ph
Fachgebiet (DDC): 621.3: Elektro-, Kommunikations-, Steuerungs- und Regelungstechnik
Zusammenfassung: Numerical modeling of proton exchange membrane fuel cells is at the verge of becoming predictive. A crucial requisite for this, though, is that material properties of the membrane-electrode assembly and their functional dependence on the conditions of operation are known with high precision. In this bipartite paper series we determine the most critical transport parameters for which accurate experimental characterization is required in order to enable the simulation of fuel cell operation with sufficient confidence from small to large current densities. In Part II, we employ the two-phase model developed in Part I to carry out extensive forward uncertainty propagation analyses. These include the study of local parameter sensitivity in the vicinity of a baseline parameter set, and a global sensitivity analysis in which a broad range of operating conditions and material properties is covered. A comprehensive ranking list of model parameters is presented, sorted by impact on predicted fuel cell properties such as the current-voltage characteristics and water balance. The top five in this list are, in this order: The membrane hydration isotherm, the electro-osmotic drag coefficient, the membrane thickness, the water diffusivity in the ionomer and its ionic conductivity.
URI: https://digitalcollection.zhaw.ch/handle/11475/17089
Volltext Version: Akzeptierte Version
Lizenz (gemäss Verlagsvertrag): CC BY-NC-ND 4.0: Namensnennung - Nicht kommerziell - Keine Bearbeitungen 4.0 International
Gesperrt bis: 2021-05-03
Departement: School of Engineering
Organisationseinheit: Institute of Computational Physics (ICP)
Publiziert im Rahmen des ZHAW-Projekts: SCCER-Mobility
Enthalten in den Sammlungen:Publikationen School of Engineering

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Vetter, R., & Schumacher, J. O. (2019). Experimental parameter uncertainty in proton exchange membrane fuel cell modeling - part II : sensitivity analysis and importance ranking. Journal of Power Sources, 439, 126529. https://doi.org/10.1016/j.jpowsour.2019.04.057
Vetter, R. and Schumacher, J.O. (2019) ‘Experimental parameter uncertainty in proton exchange membrane fuel cell modeling - part II : sensitivity analysis and importance ranking’, Journal of Power Sources, 439, p. 126529. Available at: https://doi.org/10.1016/j.jpowsour.2019.04.057.
R. Vetter and J. O. Schumacher, “Experimental parameter uncertainty in proton exchange membrane fuel cell modeling - part II : sensitivity analysis and importance ranking,” Journal of Power Sources, vol. 439, p. 126529, Nov. 2019, doi: 10.1016/j.jpowsour.2019.04.057.
VETTER, Roman und Jürgen O. SCHUMACHER, 2019. Experimental parameter uncertainty in proton exchange membrane fuel cell modeling - part II : sensitivity analysis and importance ranking. Journal of Power Sources. 1 November 2019. Bd. 439, S. 126529. DOI 10.1016/j.jpowsour.2019.04.057
Vetter, Roman, and Jürgen O. Schumacher. 2019. “Experimental Parameter Uncertainty in Proton Exchange Membrane Fuel Cell Modeling - Part II : Sensitivity Analysis and Importance Ranking.” Journal of Power Sources 439 (November): 126529. https://doi.org/10.1016/j.jpowsour.2019.04.057.
Vetter, Roman, and Jürgen O. Schumacher. “Experimental Parameter Uncertainty in Proton Exchange Membrane Fuel Cell Modeling - Part II : Sensitivity Analysis and Importance Ranking.” Journal of Power Sources, vol. 439, Nov. 2019, p. 126529, https://doi.org/10.1016/j.jpowsour.2019.04.057.


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