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Please use this identifier to cite or link to this item: https://doi.org/10.21256/zhaw-30341
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dc.contributor.authorShin, Bong‐Rim-
dc.contributor.authorYu, In Cheol-
dc.contributor.authorPuc, Uros-
dc.contributor.authorKim, Won Tae-
dc.contributor.authorYoon, Woojin-
dc.contributor.authorKim, Chaeyoon-
dc.contributor.authorYun, Hoseop-
dc.contributor.authorKim, Dongwook-
dc.contributor.authorJazbinsek, Mojca-
dc.contributor.authorRotermund, Fabian-
dc.contributor.authorKwon, O‐Pil-
dc.date.accessioned2024-03-22T10:39:46Z-
dc.date.available2024-03-22T10:39:46Z-
dc.date.issued2023-07-03-
dc.identifier.issn2195-1071de_CH
dc.identifier.urihttps://digitalcollection.zhaw.ch/handle/11475/30341-
dc.description.abstractDevelopment of new organic crystals possessing large second-order optical nonlinearity is very challenging because of strong tendency of centrosymmetric dipole–dipole molecular assembly in crystals. This tendency makes it difficult to develop various analogous crystals that allow fine tuning of optical and physical properties to enhance the device performance. A design approach of an isomorphic crystal library consisting of 11 highly efficient nonlinear optical salt crystals is reported. Analyzing the so-called isomorphic tolerance space in previously reported mother crystals (PMnXQ chromophores, where PM denotes piperidin-4-ylmethanol electron donor, n corresponds to the substi-tuted position of halogen (X) group on the quinolinium (Q) electron acceptor), various substituents are introduced into the PMnXQ crystals at different posi-tions, considering their space-filling characteristics and interionic interaction ability. All 11 PMnXQ crystals exhibit an isomorphic (or pseudo-isomorphic) crystal structure, in which the cationic chromophores form a perfectly parallel assembly for maximizing the second-order nonlinear optical susceptibility. The optical, physical, and crystal characteristics of newly designed, synthesized, and grown isomorphic PMnXQ crystals show both similarities and differences. Excellent THz wave-generation performance is demonstrated in both kHz- and MHz-repetition optical pump systems with new PMnXQ crystals. Therefore, the design approach using isomorphic tolerance space is very attractive for developing diverse isomorphic analogous organic crystals.de_CH
dc.language.isoende_CH
dc.publisherWileyde_CH
dc.relation.ispartofAdvanced Optical Materialsde_CH
dc.rightsLicence according to publishing contractde_CH
dc.subjectNonlinear opticsde_CH
dc.subjectTerahertz wavede_CH
dc.subjectOrganic crystalde_CH
dc.subjectTHz photonicsde_CH
dc.subject.ddc621.3: Elektro-, Kommunikations-, Steuerungs- und Regelungstechnikde_CH
dc.titleDesign and validation of isomorphic crystal library for nonlinear optics and THz wave generationde_CH
dc.typeBeitrag in wissenschaftlicher Zeitschriftde_CH
dcterms.typeTextde_CH
zhaw.departementSchool of Engineeringde_CH
zhaw.organisationalunitInstitute of Computational Physics (ICP)de_CH
dc.identifier.doi10.1002/adom.202201420de_CH
dc.identifier.doi10.21256/zhaw-30341-
zhaw.funding.euNode_CH
zhaw.issue13de_CH
zhaw.originated.zhawYesde_CH
zhaw.pages.start2201420de_CH
zhaw.publication.statusacceptedVersionde_CH
zhaw.volume11de_CH
zhaw.embargo.end2024-10-26de_CH
zhaw.publication.reviewPeer review (Publikation)de_CH
zhaw.funding.snf188194de_CH
zhaw.webfeedPhotonicsde_CH
zhaw.author.additionalNode_CH
zhaw.display.portraitYesde_CH
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Shin, B.-R., Yu, I. C., Puc, U., Kim, W. T., Yoon, W., Kim, C., Yun, H., Kim, D., Jazbinsek, M., Rotermund, F., & Kwon, O.-P. (2023). Design and validation of isomorphic crystal library for nonlinear optics and THz wave generation. Advanced Optical Materials, 11(13), 2201420. https://doi.org/10.1002/adom.202201420
Shin, B.-R. et al. (2023) ‘Design and validation of isomorphic crystal library for nonlinear optics and THz wave generation’, Advanced Optical Materials, 11(13), p. 2201420. Available at: https://doi.org/10.1002/adom.202201420.
B.-R. Shin et al., “Design and validation of isomorphic crystal library for nonlinear optics and THz wave generation,” Advanced Optical Materials, vol. 11, no. 13, p. 2201420, Jul. 2023, doi: 10.1002/adom.202201420.
SHIN, Bong‐Rim, In Cheol YU, Uros PUC, Won Tae KIM, Woojin YOON, Chaeyoon KIM, Hoseop YUN, Dongwook KIM, Mojca JAZBINSEK, Fabian ROTERMUND und O‐Pil KWON, 2023. Design and validation of isomorphic crystal library for nonlinear optics and THz wave generation. Advanced Optical Materials. 3 Juli 2023. Bd. 11, Nr. 13, S. 2201420. DOI 10.1002/adom.202201420
Shin, Bong‐Rim, In Cheol Yu, Uros Puc, Won Tae Kim, Woojin Yoon, Chaeyoon Kim, Hoseop Yun, et al. 2023. “Design and Validation of Isomorphic Crystal Library for Nonlinear Optics and THz Wave Generation.” Advanced Optical Materials 11 (13): 2201420. https://doi.org/10.1002/adom.202201420.
Shin, Bong-Rim, et al. “Design and Validation of Isomorphic Crystal Library for Nonlinear Optics and THz Wave Generation.” Advanced Optical Materials, vol. 11, no. 13, July 2023, p. 2201420, https://doi.org/10.1002/adom.202201420.


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