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  2. School of Engineering
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  4. Publikationen School of Engineering
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dc.contributor.authorKim, Seung-Jun-
dc.contributor.authorYu, In Cheol-
dc.contributor.authorLee, Ji-Ah-
dc.contributor.authorKim, Won Tae-
dc.contributor.authorJazbinsek, Mojca-
dc.contributor.authorYoon, Woojin-
dc.contributor.authorYun, Hoseop-
dc.contributor.authorRotermund, Fabian-
dc.contributor.authorKwon, O-Pil-
dc.date.accessioned2022-03-01T15:21:30Z-
dc.date.available2022-03-01T15:21:30Z-
dc.date.issued2021-08-
dc.identifier.issn0143-7208de_CH
dc.identifier.urihttps://digitalcollection.zhaw.ch/handle/11475/24344-
dc.description.abstractIn this study, we develop new organic benzothiazolium crystals possessing very large off-diagonal optical nonlinearity. In these crystals, benzothiazolium-based 2-(4-(4-(hydroxymethyl)piperidin-1-yl)styryl)-3-methyl-benzothiazol-3-ium (PMB) cations with large molecular optical nonlinearity are incorporated with two anions: 4 (trifluoromethoxy)benzenesulfonate (TFO) with an orthogonal non-planar shape and 5-bromothiophene-2-sulfonate (BTS) with a planar shape. Both PMB-TFO and PMB-BTS crystals exhibit state-of-the-art off-diagonal effective hyperpolarizability that results from the V-shape and X-shape alignments of PMB chromophores, respectively. Newly developed PMB crystals indicate excellent characteristics for second-order nonlinear optical applications such as difference-frequency generation (e.g. optical rectification) and sum-frequency generation (e.g. second-harmonic generation), which are comparable to current benchmark organic crystals.de_CH
dc.language.isoende_CH
dc.publisherElsevierde_CH
dc.relation.ispartofDyes and Pigmentsde_CH
dc.rightsLicence according to publishing contractde_CH
dc.subjectTHz photonicsde_CH
dc.subjectOrganic crystalde_CH
dc.subjectNonlinear opticsde_CH
dc.subjectElectro-opticsde_CH
dc.subject.ddc621.3: Elektro-, Kommunikations-, Steuerungs- und Regelungstechnikde_CH
dc.titleNew benzothiazolium crystals with very large off-diagonal optical nonlinearityde_CH
dc.typeBeitrag in wissenschaftlicher Zeitschriftde_CH
dcterms.typeTextde_CH
zhaw.departementSchool of Engineeringde_CH
zhaw.organisationalunitInstitute of Computational Physics (ICP)de_CH
dc.identifier.doi10.1016/j.dyepig.2021.109433de_CH
zhaw.funding.euNode_CH
zhaw.issue109433de_CH
zhaw.originated.zhawYesde_CH
zhaw.publication.statuspublishedVersionde_CH
zhaw.volume192de_CH
zhaw.publication.reviewPeer review (Publikation)de_CH
zhaw.funding.snf188194de_CH
zhaw.webfeedPhotonicsde_CH
zhaw.funding.zhawMolecular Phonon-Mode Engineering for All-Organic Gap-Free THz Photonicsde_CH
zhaw.author.additionalNode_CH
zhaw.display.portraitYesde_CH
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Kim, S.-J., Yu, I. C., Lee, J.-A., Kim, W. T., Jazbinsek, M., Yoon, W., Yun, H., Rotermund, F., & Kwon, O.-P. (2021). New benzothiazolium crystals with very large off-diagonal optical nonlinearity. Dyes and Pigments, 192(109433). https://doi.org/10.1016/j.dyepig.2021.109433
Kim, S.-J. et al. (2021) ‘New benzothiazolium crystals with very large off-diagonal optical nonlinearity’, Dyes and Pigments, 192(109433). Available at: https://doi.org/10.1016/j.dyepig.2021.109433.
S.-J. Kim et al., “New benzothiazolium crystals with very large off-diagonal optical nonlinearity,” Dyes and Pigments, vol. 192, no. 109433, Aug. 2021, doi: 10.1016/j.dyepig.2021.109433.
KIM, Seung-Jun, In Cheol YU, Ji-Ah LEE, Won Tae KIM, Mojca JAZBINSEK, Woojin YOON, Hoseop YUN, Fabian ROTERMUND und O-Pil KWON, 2021. New benzothiazolium crystals with very large off-diagonal optical nonlinearity. Dyes and Pigments. August 2021. Bd. 192, Nr. 109433. DOI 10.1016/j.dyepig.2021.109433
Kim, Seung-Jun, In Cheol Yu, Ji-Ah Lee, Won Tae Kim, Mojca Jazbinsek, Woojin Yoon, Hoseop Yun, Fabian Rotermund, and O-Pil Kwon. 2021. “New Benzothiazolium Crystals with Very Large Off-Diagonal Optical Nonlinearity.” Dyes and Pigments 192 (109433). https://doi.org/10.1016/j.dyepig.2021.109433.
Kim, Seung-Jun, et al. “New Benzothiazolium Crystals with Very Large Off-Diagonal Optical Nonlinearity.” Dyes and Pigments, vol. 192, no. 109433, Aug. 2021, https://doi.org/10.1016/j.dyepig.2021.109433.


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